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자료유형
학술저널
저자정보
저널정보
한국대기환경학회 한국대기환경학회지(국문) 한국대기환경학회지 제20권 제4호
발행연도
2004.8
수록면
555 - 569 (15page)

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Size-segregated measurements of aerosol composition using X-stage DRUM impactor are used to determine the transport of natural and anthropogenic aerosols at Gosan site from 29 March to 30 May in 2002. Separation of ambient aerosols by DRUM impactor offers many advantages over other standard filtration techniques. Some of the most important advantages are the ability to segregate into details by particle size, to better preserve chemical integrity since the air stream doesn't pass through the deposit, to collect samples as a function of time, and to have a wide variety of impaction surfaces available to match analytical needs.
Although the transport of Yellow sand is a well-known phenomenon in springtime, the result of measurement shows that not only soil dust but also anthropogenic aerosols, including sulfur, enriched trace metals such as Pb, Ni, Zn, Cu, Cr, As, Se, Hr, are transported to Gosan in springtime. This study combines the size- and time- resolved aerosol composition measurements with isentropic, backward air-mass trajectories in order to identify some potential source regions of anthropogenic aerosols. As a result, during the NYS period, the average concentration of PM_10 was 46 ㎍/㎥. Si, Al, S, Fe, Cl, K, Ca were higher than 1,000 ㎍/㎥ and Ti was about 100 ㎍/㎥. The concentrations of Zn, Mn, Cu, Pb, Br, Rb, V, Cr, Ni, As, Se ranged between 1 and 70 ㎍/㎥. More than 50% of typical soil elements, such as Al, Si, Fe, Ca, Ti, Cr, Cu, Br, were distributed in a coarse particle range (5.0 ~ 12μm). In other hand, anthropogenic pollutants, such as S, N, Vi, were mainly distributed in a fine particle range (0.09 ~ 0.56μm). During the YS period, PM_10 increased about 8 times than NYS period, and main soil elements, such as Al, Si, S, K, V, Mn, Fe also doubled in coarse particle range (1.15 ~ 12μm). But Zn, As, Pb, Cu and Se, which distributed in the fine aerosols (0.09 ~0.56μm), were on the same level with or decreased than NYS period. Finally, except the YS period, coarse particles (2.5 ~ 12μm) arc inferred to be influenced by soil, coal combustion, waste incineration, ferrous and nonferrous sources through similar pathways with Yellow Sand. But line particles have different sources, such as coal combustion, gasoline vehicle, biomass burning, oil or coal combustion, nonferrous and ferrous metal sources, which are transported from China, Korea peninsula and local sources.

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UCI(KEPA) : I410-ECN-0101-2009-539-014260887