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논문 기본 정보
- 자료유형
- 학술저널
- 저자정보
- 발행연도
- 2015.1
- 수록면
- 867 - 874 (8page)
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Separation of cesium chloride (CsCl) and strontium chloride (SrCl2) from the lithiumchloride-potassium chloride (LiCl-KCl) salt was studied using a melt crystallization processsimilar to the reverse vertical Bridgeman growth technique. A ternary SrCl2-LiCl-KCl saltwas explored at similar growth rates (1.8e5 mm/h) and compared with CsCl ternary resultsto identify similarities. Quaternary experiments were also conducted and compared withthe ternary cases to identify trends and possible limitations to the separations process. Inthe ternary case, as much as 68% of the total salt could be recycled per batch process. In thequaternary experiments, separation of Cs and Sr was nearly identical at the slower rates;however, as the growth rate increased, SrCl2 separated more easily than CsCl. The quaternaryresults show less separation and rate dependence than in both ternary cases. As anestimated result, only 51% of the total salt could be recycled per batch. Furthermore, twomodels have been explored to further understand the growth process and separation. Acomparison of the experimental and modeling results reveals that the nonmixed model fitsreasonably well with the ternary and quaternary data sets. A dimensional analysis wasperformed and a correlation was identified to semipredict the segregation coefficient.
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참고문헌 (16)
참고문헌 신청
A.N. Wiliams / 2012 / Zone Freezing Study for Pyrochemical Process Waste Minimization / 석사 / University of Idaho
A.N. Williams / 2013 / Separation of CsCl from a ternary CsCl-LiCl-KCl salt via a melt crystallization technique for pyroprocessing waste minimization / Chem. Eng. Sci 89 :
E. Scheil / 1931 / Bemerkungen zur schichtkristall bildung / Z. Metallkd 23 : 237 ~
J. Ackerman / 1997 / Treatment of wastes in the IFR fuel cycle / Prog. Nucl. Energy 31 : 141 ~ 154
J. Choi / 2013 / Inclusion behavior of Cs, Sr, and Ba impurities in LiCl crystal formed by layer-melt crystallization: combined firstprinciples calculation and experimental
A.N. Williams / 2013 / Separation of CsCl from a ternary CsCl-LiCl-KCl salt via a melt crystallization technique for pyroprocessing waste minimization / Chem. Eng. Sci 89 :
E. Scheil / 1931 / Bemerkungen zur schichtkristall bildung / Z. Metallkd 23 : 237 ~
J. Ackerman / 1997 / Treatment of wastes in the IFR fuel cycle / Prog. Nucl. Energy 31 : 141 ~ 154
J. Choi / 2013 / Inclusion behavior of Cs, Sr, and Ba impurities in LiCl crystal formed by layer-melt crystallization: combined firstprinciples calculation and experimental
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